Time delay in valence shell photoionization of noble gas atoms

نویسنده

  • A. S. Kheifets
چکیده

We use the non-relativistic random phase approximation with exchange to perform calculations of valence shell photoionization of Ne, Ar, Kr and Xe from their respective thresholds to photon energy of 200 eV. The energy derivative of the complex phase of the photoionization matrix elements is converted to the photoelectron group delay that can be measured in attosecond streaking or twophoton transitions interference experiments. Comparison with reported time delay measurements in Ne and Ar at a few selected photon energies is made. Systematic mapping of time delay across a wide range of photon energies in several atomic targets allows to highlight important aspects of fundamental atomic physics that can be probed by attosecond time delay measurements.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Nondipole Effects in Photoionization of Rare Gas Atoms

We present a discussion of octupole and other O(k2) (k = 2π/λ, where λ is the photon wavelength) corrections to to the angular distribution of photoelectrons from noble-gas atoms. These corrections are characterized by four parameters ∆β, λ, μ, and ν constrained by λ+μ+ν = 0. As an example, we consider photoionization of n = 2 shell of neon for photon energies below 2 keV. The resulting angular...

متن کامل

Theoretical Auger and photoionization studies for open-shell atoms and ions

In the last few years, the RATIP package has been found useful for studying the properties of atoms and (highly charged) ions within rather arbitrary configurations. Here, the latest extensions to this code are reviewed which help calculate several Auger and photoionization parameters, including cross sections, angular coefficients as well as correlation functions for the emitted electrons. In ...

متن کامل

Positronium formation from valence and inner shells in noble gas atoms

When recent experimental positronium (Ps) formation cross sections in noble gases have been compared with the most up-to date theoretical studies, the agreement is qualitative, but not quantitative. In this paper we re-examine this process and show that at low energies Ps formation must be treated nonperturbatively. We also look at Ps formation with inner shell electrons.

متن کامل

Photoionization of helium nanodroplets doped with rare gas atoms.

Photoionization of He droplets doped with rare gas atoms (Rg=Ne, Ar, Kr, and Xe) was studied by time-of-flight mass spectrometry, utilizing synchrotron radiation from the Advanced Light Source from 10 to 30 eV. High resolution mass spectra were obtained at selected photon energies, and photoion yield curves were measured for several ion masses (or ranges of ion masses) over a wide range of phot...

متن کامل

K(h)α1,2 x-ray hypersatellite line broadening as a signature of K-shell double photoionization followed by outer-shell ionization and excitation.

We propose a novel approach for the theoretical analysis of the photoinduced high-resolution K(h)α(1,2) x-ray hypersatellite spectra, which allows us to obtain reliable values of lifetimes of the doubly K-shell ionized states and fundamental information about the relative role of K-shell double photoionization (DPI) mechanisms. It is demonstrated for the first time that the K(h)α(1,2) hypersate...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

عنوان ژورنال:

دوره   شماره 

صفحات  -

تاریخ انتشار 2012